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Lim Lab

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Tsong-Shin Lim
Associate Professor
Department of Applied Physics
Tunghai University
TEL:+886-4-2359-0121 ext.32116
Fax: 886-4-2359-4643
Cellular phone:+886-952-006340
Email: tslim@thu.edu.tw
No.1727, Sec.4, Taiwan Boulevard, Xitun District, Taichung City 407224, Taiwan R.O.C.


Education

Ph. D. -- Department of physics, National Cheng Kung University 1998/9-2001/11
M. S. -- Department of Physics, National Cheng Kung University 1996/9-1998/7
B. S. -- Department of Physics, National Cheng Kung University 1992/9-1996/7

Professional Appointments

Assistant Professor -- Department of Physics, Tunghai University 2007/8-
Postdoctoral Fellow -- Institute of Atomic and Molecular Sciences, Academia Sinica 2002/10-2007/7
Postdoctoral Fellow -- Department of Physics, National Cheng Kung University 2002/1-2002/6

Research interests

Single-molecule spectroscopy
Laser Dynamics
Bio-Physics

Publication

Journal Paper

[52]Chih-Hsien Chen, Zi-Huan Luo, I-Hong Huan, Yu-Han Chen, Tsong-Shin Lim, Rationalize the roles of electron donating-withdrawing groups in the impacts on solvatochromism, nonlinear optics, and electroluminescence devices., DYES AND PIGMENTS 175, 108143 (2020).[PDF]

[51]Eric H. -L. Chen, Tony T. -Y. Lu, Jack C. -C. Hsu, Yufeng Jane Tseng, T. -S. Lim, and Rita P. -Y. Chen, Directly monitor protein rearrangement on a nanosecond-to-millisecond time-scale, Scientific Reports 7, 8691 (2017).[PDF]

[50]Yi-Chung Dzeng, Chi-Ling Huang, Yi-Hung Liu, Tsong-Shin Lim, I-Chia Chen, Tien-Yau Luh, Substituent-Dependent Photophysical Properties Due to the Thorpe-Ingold Effect on Foldings of Alternating Substituted Methylene- Diethynylbenzene Copolymers: A Comparison of Carbon versus Silicon Tethers, Macromolecules 48, 8708-8717 (2015).[PDF]

[49]C.-W. Chen, K. Fan, C.-H. Chen, S.-L. Huang, Y.-H. Liu, T.-S. Lim, G. W. Wang, and T.-Y. Luh, Stereoselective Iterative Convergent Synthesis of Z-Oligodiacetylenes from Propargylic Dithioacetals, Journal of Organic Chemistry 80, 8772-8781 (2015).[PDF]

[48]J. C.-C. Hsu, E. H.-L. Chen, R. C. Snoeberger, F. Y. Luh, T.-S. Lim, C. P. Hsu, R. P. -Y. Chen, Thioflavin T and Its Photoirradiative Derivatives: Exploring Their Spectroscopic Properties in the Absence and Presence of Amyloid Fibrils, Journal of Physical Chemistry B 117, 3459-3468 (2013).[PDF]

[47]W.-C. Liao, W.-H. Chen, C.-H. Chen, T.-S. Lim, T.-Y. Luh, Photoinduced Electron Transfer as a Probe for the Folding Behavior of Dimethylsilylene-Spaced Alternating Donor-Acceptor Oligomers and Polymers, Macromolecules 46, 1305-1311 (2013).[PDF]

[46] Lun-Hsuan Chen, T.-S. Lim, and Huan-Cheng Chang, Measuring the number of (N-V)- centers in single fluorescent nanodiamonds in the presence of quenching effects, Journal of the Optical Society of America B 29, 2309 (2012).[PDF]

[45] L. L. Yang, M. W. P. Kao, H.-L. Chen, T.-S. Lim, W. Fann, R. P. Y. Chen, Observation of protein folding/unfolding dynamics of ubiquitin trapped in agarose gel by single-molecule FRET, European Biophysics Journal with Biophysics Letters 41, 189 (2012).[PDF]

[44] C.-H. Chen, Y. C. Huang, W. C. Liao, T.-S. Lim, K. L. Liu, I. C. Chen, and T. Y. Luh, Controlling Conformations in Alternating Dialkylsilylene-Spaced Donor-Acceptor Copolymers by a Cooperative Thorpe-Ingold Effect and Polymer Folding, Chemistry- A European Journal 18, 334 (2012).[PDF]

[43] C.-H. Chen, W. H. Chen, Y. H. Liu, T.-S. Lim, T. Y. Luh, Folding of Alternating Dialkylsilylene-Spaced Donor-Acceptor Copolymers: The Oligomer Approach, Chemistry- A European Journal 18, 347 (2012).[PDF]

[42] M.-J. Kao, C.-H. Chen, P.-Y. Tsai, T.-S. Lim, K.-C. Lin, and T.-Y. Luh, Hydrogen-Bonding-Induced One-Handed Helical Polynorbornenes Appended With Chiral Alanine, Macromolecular Chemistry and Physics 212, 2328 (2011).[PDF]

[41] C.-H. Chen, S.-L. Lee, T.-S. Lim, C.-H. Chen, and T.-Y. Luh, Influence of polymer conformations on the aggregation behaviour of alternating dialkylsilylene-[4,4'-divinyl(cyanostilbene)] copolymers, Polymer Chemistry 2, 2850 (2011).[PDF]

[40] Y.-Y. Hui, Y.-R. Chang, N. Mohan, T.-S. Lim, Y.-Y. Chen, H.-C. Chang, Polarization Modulation Spectroscopy of Single Fluorescent Nanodiamonds with Multiple Nitrogen Vacancy Centers, Journal of Physical Chemistry A 115, 1878 (2011).[PDF]

[39] H.-W. Wang, C.-H. Chen, T.-S. Lim, S.-L. Huang, T.-Y. Luh, Supramolecular Porphyrin-DABCO Array in Single- and Double-Stranded Polynorbornenes, Chemistry-an Asian Journal 6, 524 (2011).[PDF]

[38] C.-C. Fu, C.-F. Lin, Q.-Z Gao, W.-Z. Yang, T.-S. Lim, L.-L. Yang, C.-F. Yen, W.-H. Chang, H. S. Yuan, S.-Y. Sheu, D.-Y. Yang, W. Fann, Fis-protein induces rod-like DNA bending, Chemical Physics Letters 500, 318 (2010).[PDF]

[37] J. J. Liang, J. H. Hsu, T.-S. Lim, J. D. White, Photophysics of Single PPV Derivative Polymers, Journal of the Chinese Chemical Society 57, 478 (2010).[PDF]

[36] C. Y. Lo, C. H. Chen, T. W. T. Tsai, L. Zhang, T.-S. Lim, W. Fann, J. C. C. Chan, C. C. Jerry, T. Y. Luh, Efficient Energy and Electron Transfer between Donor and Acceptor Chromophores in Aluminophosphate Hybrid Materials, Journal of the Chinese Chemical Society 57, 539 (2010).[PDF]

[35] Z. C. Liu, C. H. Chen, H. W. Wang, Y. C. Huang, M. J. Kao, T.-S. Lim, T. Y. Luh, Hydrogen-Bonding Induced Cooperative Effect on the Energy Transfer in Helical Polynorbornenes Appended with Porphyrin-Containing Amidic Alanine Linkers, Chemistry-an Asian Journal 5, 1425 (2010).[PDF]

[34] K. W. Yang, J. Xu, C. H. Chen, H. H. Huang, T. J.-Y. Yu, T.-S. Lim , C. H. Chen, T. Y. Luh, Triple-Stranded Polymeric Ladderphanes, Marcomolecules 43, 5188 (2010). [PDF]

[33] C.M. Chou, C.H. Chen, C.L. Lin, K.W. Yang, T.-S. Lim, T.Y. Luh, Alternating furanylene-meta-phenylene oligomers: synthesis and photophysics, Tetrahedron 65, 9749 (2009). [PDF]

[32] A. Rassamesard, Y.F. Huang, H.Y. Lee, T.-S. Lim, M.C. Li, J.D. White, J.H. Hodak, T. Osotchan, K.Y. Peng, S.A. Chen, J.H. Hsu, M. Hayashi, W. Fann,Environmental Effect on the Fluorescence Lifetime and Quantum Yield of Single Extended Luminescent Conjugated Polymers, Journal of Physical Chemistry C 113, 18681 (2009). [PDF]

[31] C.M. Chou, S.L. Lee, C.H. Chen, A.T. Biju, H.W. Wang, Y.L. Wu, G.F. Zhang, K.W. Yang, T.-S. Lim, M.J. Huang, P.Y. Tsai, K.C. Lin, S.L. Huang, C.H. Chen, T.Y. Luh, Polymeric Ladderphanes, Journal of the American Chemical Society 131, 35 (2009). [PDF]

[30] Y.-F. Huang, C.W. Chang, D.M. Smilgies, U.S. Jeng, A.R. Inigo, J.D. White, K.C. Li, T.-S. Lim, T.D. Li, H.Y. Chen, S.A. Chen, W.C. Chen, W.S. Fann, Correlating Nanomorphology with Charge-Transport Anisotropy in Conjugated-Polymer Thin Films, Advanced Materials 21, 2988 (2009). [PDF]

[29] H. L. Chen, Y. F. Huang, T.-S. Lim, C. H. Su, P. H. Chen, A. C. Su, K. T. Wong, T. C. Chao, S. I. Chan, and W. Fann, Excited-State Backbone Twisting of Polyfluorene As Detected from Photothermal After-Effects, Journal Physial Chemistry B 113, 8527 (2009). [PDF]

[28] H.-W. Wang, Z.-C. Liu, C.-H. Chen, T.-S. Lim, W. Fann, C.-G. Chao, J.-Y. Yu, S.-L. Lee, C.-H. Chen, S.-L. Huang, and T.-Y. Luh, Coherently Aligned Porphyrin-Appended Polynorbornenes, Chemistry - A European Journal 15, 5719 (2009). [PDF]

[27] T.-S. Lim, C. C. Fu, K. C. Lee, H. Y. Lee, K. Chen, W. F. Cheng, W.W. Pai, H. C. Chang, and W. Fann, Fluorescence enhancement and lifetime modification of single nanodiamonds near a nanocrystalline silver surface, Physical Chemistry Chemical Physics 11, 1508 (2009). [PDF]

[26] Evan S.-H. Chang, Tai-Yan Liao, T.-S. Lim, W. Fann, Rita P.-Y. Chen, A New Amyloid-Like beta-Aggregate with Amyloid Characteristics, Except Fibril Morphology, Journal of Molecular Biology 385, 1257 (2009). [PDF]

[25] Yuen Yung Hui, Yi-Ren Chang, T.-S. Lim, Hsu-Yang Lee, Wunshain Fann, Huan-Cheng Chang, Quantifying the number of color centers in single fluorescenct nanodiamonds by photon correlation spectroscopy and Monte Carlo simulation, Applied Physics Letters 94, 013104 (2009). [PDF]

[24] Michael Wen-Pin kao, Li-Ling Yang, Jacky Chih-Kai Lin, T.-S. Lim, Wunshain Fann, Rita P. -Y. Chen, Strategy for efficient site-specific FRET-dye labeling of ubiquitin, Bioconjugate Chemistry 19, 1124 (2008). [PDF]

[23] Yi-Ren Chang, Hsu-Yang Lee, Kowa Chen, Chun-Chieh Chang, Dung-Sheng Tsai, Chi-Cheng Fu, T.-S Lim, Yan-Kai Tzeng, Chia-Yi Fang, Chau-Chung Han, Huan-Cheng Chang, Wunshain Fann, Mass production and dynamic imaging of fluorescent nanodiamonds, Nature Nanotechnology 3, 284 (2008). [PDF]

[22] H. W. Wan, M. Y. Yeh, C. H. Chen, T.-S. Lim, W Fann, and T. Y. Luh, Coupling of FRET and photoinduced electron transfer in regioregular silylene-spaced energy donor-acceptor-electron donor copolymers, Marcomolecules 41, 2762 (2008). [PDF]

[21] C. L. Lin, C. H. Chen, T.-S. Lim, W Fann, and T. Y. Luh, Combining Light Harvesting and Electron Transfer in Silica-titania-based Organic-inorganic Hybrid Materials, Chemistry-an Asian Journal 3, 578 (2008). [PDF]

[20] M. Y. Yeh, H. C. Lin, T.-S. Lim, S. L. Lee, C. H. Chen, W.Fann, and T. Y. Luh, Thorpe-Ingold Effect on Photoinduced Electron Transfer of Dialkylsilylene-spaced Divinylarene Copolymers Having Alternating Donor and Acceptor Chromophores, Macromolecules 40, 9238 (2007). [PDF]

[19] Y. F. Huang, A. R. Inigo, C. C. Chang, K. C. Li, C. F. Liang, C. W. Chang, T.-S. Lim, S. H. Chen, J. D. White, U. S. Jeng, A. C. Su, Y. S. Huang, K. Y. Peng, S. A. Chen, W. W. Pai, C. H. Lin, A. R. Tameev, S. V. Novikov, A. V. Vannikov, and W. S. Fann, Nanostructure-dependent Vertical Charge Transport in MEH-PPV Films, Advanced Functional Materials 17, 2902 (2007). [PDF]

[18] M.-Y. Yeh, H.-C. Lin, S.-L. Lee, C.-h. Chen, T.-S. Lim, W. Fann, and T.-Y. Luh, Thorpe¡VIngold Effect on the Conformation and Photophysical Properties of Dialkylsilylene-spaced Divinylarene Copolymers, Chemical Communications, 3459 (2007).[PDF]

[17] Hsin-Liang Chen, Yi-Fang Huang, Chao-Ping Hsu, T.-S. Lim, Li-Chung Kuo, Man-kit. Leung, Teng-Chih Chao, Ken-Tsung Wong, Show-An Chen, and Wunshain Fann, Direct Measurements of Intersystem Crossing Rates and Triplet Decays of Luminescent Conjugated Oligomers in Solutions, The Journal of Physical Chemistry A 111, 9424 (2007).[PDF]

[16] T.-S. Lim, J. C. Hsiang, J. D. White, W. S. Fann, Y. L. Fan, and K. F. Lin, Single Short-chain Conjugated Polymer Studied with Optical Spectroscopy: A Donor-accepter System, Physical Review B 75, 165204 (2007).[PDF]

[15] H.-W. Wang, Y.-J. Cheng, C.-H. Chen, T.-S. Lim, W. S. Fann, C.-L. Lin, Y.-P. Chang, K.-C. Lin, and T.-Y. Luh, Photoinduced Electron Transfer in Silylene-Spaced Copolymers Having Alternating Donor-Acceptor Chromophores, Macromolecules 40, 2666 (2007).[PDF]

[14] C.-C. Fu, H.-Y. Lee, K. Chen, T.-S. Lim, H. Y. Wu, P.-K. Lin, P.-K. Wei, P. H. Tsao, H.-C. Chang, and W. S. Fann, Characterization and Applications of Single Fluorescent Nanodiamonds as Cellular Biomarkers, Proceedings of the National Academy of Sciences 104, 727 (2007).[PDF]

[13] J. J. Liang, J. D. White, Y. C. Chen, C. F. Wang , J. C. Hsiang, T.-S. Lim, W. Y. Sun, J. H. Hsu, C. P. Hsu , M. Hayashi, W. S. Fann, K. Y. Peng, and S. A. Chen, Heterogeneous Energy Landscapes of Individual Luminescent Conjugated Polymers, Physical Review B 74, 085209 (2006).[PDF]

[12] C. H. Chen, K. Y. Liu, S. Sudhakar, T.-S. Lim, W. S. Fann, C. P. Hsu, and T. Y. Luh, Efficient Light Harvesting and Energy Transfer in Organic Anorganic Hybrid Multichromophoric Materials, Journal of Physical Chemistry B 109, 17887 (2005).[PDF]

[11] T.-S. Lim, J.-L. Chern, and K. Otsuka, Higher-order photon statistics of single-mode laser diodes and microchip solid-state Lasers, Optics Letters 27, 2197 (2002).[PDF]

[10] K. Otsuka, J.-Y. Ko, T.-S. Lim, and H. Makino, Modal interference and dynamical instability in a solid-state microchip laser, Physical Review Letters 89, 083903 (2002).[PDF]

[9] K. Otsuka, T.-S. Lim, J.-Y. Ko, and H. Makino, Self-induced high-speed modulation in a microchip solid-state laser with asymmetric end-pumping, Optics Letters 27, 1696 (2002).[PDF]

[8] K. Otsuka, K. Abe, J.-Y. Ko, and T.-S. Lim, Real-time nanometer-vibration measurement with a self-mixing microchip solid-state laser, Optics Letters 27, 1339 (2002). [PDF]

[7] T.-S. Lim, J.-L. Chern , and K. Otsuka, Relative Intensity Fluctuation of Single-mode Class-B Lasers, Optics Letters 27, 1037 (2002).[PDF]

[6] J.-L Chern, T. Kubota, T.-S. Lim, and K. Otsuka, Stokes-like Emissions from Laser-diode-pumped Microchip Nd-doped Solid-state Lasers, Journal of the Optical Society of America B 19, 1668 (2002). [PDF]

[5] T.-H. Yang, T.-S. Lim, J.-L. Chern, and K. Otsuka, Non-stationary characteristic of instability in a single-mode Nd:YVO4 laser with fiber feedback, European Physics Journal D 15, 365 (2001).[PDF]

[4] T.-S. Lim, T.-H. Yang, J.-L. Chern, and K. Otsuka,Phase-noise-driven Instability in a Single-mode Microchip Nd:YVO4 Laser with Feedback, IEEE Journal of Quantum Electronics 37, 1215(2001).[PDF]

[3] K. Otsuka, J.-Y. Ko, T. Kubota, S.-L. Hwong, T.-S. Lim, J.-L. Chern, B. A. Nguyen, and P. Mandel, Instability in a Laser-Diode-Pumped Microchip Nd:YAG Laser in a P-scheme, Optics Letters 26, 1060 (2001). [PDF]

[2] S.-L. Hwong, W.-L. Tsai, T.- S. Lim and J.-L. Chern, Influences of pump-beam focusing conditions on a laser-diode-pumped microchip Nd:YVO4 laser, Japanese Journal of Applied Physics Part 2-Lett. 38, L1300 (1999).

[1] Y.-F. Huang, H.-Y. Ueng, C.-R. Chung, L.-W. Tu, T.-S. Lim, W.-C. Chen, and J.-L. Chern, Complex time series from a modulated semiconductor laser: Its determinism exploration, IEEE Journal of Quantum Electronics 35, 757 (1999).[PDF]

Conference Paper

[5] T.-S. Lim, C. Fu, H. Lee, K. Chen, P. Lin, H. Wu, P. Wei, P. Tsao, H. Chang, and W. Fann, Single Fluorescent Nanodiamond: a Potential Cellular Biomarker, SPIE Photonics West 2007: Ultrasensitive and Single-molecule Detection Technologies II, 6444-01.(oral)

[4] T.-S. Lim, J.-L. Chern, and K. Otsuka, High-order photon statistics of singl-mode laser dioeds and microchip solid-state lasers, IQEC/LAT 2002, June 22-28, 2002, Moscow, Russia (oral).

[3] J.-L. Chern and T.-S. Lim, Synchronized chaos in mutually coupled Nd:YVO4 microchip lasers, CLEO/Europe-EQEC 2001, June 18-22, 2001 Munich, Germany.

[2] J.-L. Chern and T.-S. Lim, Phonon-assisted Frequency Conversion in Laser-diode pumped Nd:doped Microchip Solid State Lasers, CLEO/Europe-EQEC 2001, June 18-22, 2001, Munich, Germany.

[1] S.-L. Hwong, J.-L. Chern, T.-S. Lim, and K. Otsuka, Dynamical instability in a laser-diode-pumped multitransition-oscillation Nd:YAG laser, IQEC 2000, QWB7, September 10-15, Nice, France, 2000 (oral)

Ph. D. Thesis

Complex dynamical behaviors in LD-pumped microchip solid-state lasers
Department of Physics, National Cheng Kung University December 2001
Superviser: Professor Jyh-Long Chern

M. S. Thesis

Study on the stochastic response around transcritical bifurcation and its experimental counterpart in semiconductor lasers
Department of Physics, National Cheng Kung University July 1998
Superviser: Porfessor Jyh-Long Chern
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